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This research aims to develop a module of medicinal plants for subject organic chemistry in natural materials to stimulate the metacognitive skills of students Tadris IPA IAIN Bengkulu. The research method refers to the steps of Research and Development. The research is began by analyzing the needs of subject organic chemistry in natural and plant materials that are often used by Bengkulu people as medicines to be used as learning resources in the form of modules. The trial of module was limited to 16 students of semester IV in the IAIN Bengkulu, Natural Sciences Study Program. The results showed that the metacognitive skills of students using the medicinal herbs module varied greatly. Student metacognitive skills are mostly good (50%), very good (6%), sufficient (6%), and lacking (38%). The ability of students in the planning aspect has developed well while the aspects of monitoring, evaluating, and revising have not developed well (enough). This local potential medicinal plant module is able to stimulate the metacognitive abilities of the fourth semester students, Tadris natural sciences Study Program, IAIN Bengkulu viewed from the classical values.