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E-learning is distance learning that utilized computer technology, computer networks and/or internet networks. To produce an innovative learning process, an innovative learning media is also needed, namely edmodo media. The purpose of this study is to describe the validity of innovative learning tools based on e-learning with edmodo to improve high-level thinking skills (HOTS). Data validity was obtained through expert valization and forum group discussion (FGD) conducted with assesment, suggestion and consideration through expert validation sheets. The results obtained from expert validation and FGD obtained from research and development include the following : (1) the validity of e-learning and edmodo based innovative learning devices to improve high-level thinking skills declared valid with some suggestions and input; (2) validation of innovative e-learning based learning models with edmodo to improve high-level thinking skills declared valid with some suggestions and input. Based on the results of research and development, it can be concluded that the e-learning based learning tool with edmodo to improve high-level thinking skills is declared valid to be used in the process of learning activities