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Education and technology must run together in this millenial century. This study aims to develop teaching materials based on mobile learning for thematic learning in elementary school. This study uses research and development methods by Dick and Carey model. The instruments used in this study were interviews, questionnaires, and tests. The result of this study are teaching materials based on mobile learning. Based on the results of the pre-test and post-test analysis, it showed that there were differences in learning outcomes between the pre-test and post-test stages. The results of the t-test show that t count = 12.10 and t table = 1.99 at the significance level α = 0.05 / 95%. Thus it can be concluded that there is an increase in learning outcomes experienced by students, after participating in thematic learning with teaching materials based on mobile learning.